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Life cycle assessment of ibuprofen removal by advanced oxidation processes

Yıl 2021, Sayı: 28, 795 - 801, 30.11.2021

Öz

Ibuprofen (IBU), which is in the non-steroidal anti-inflammatory (NSAI) group, is frequently detected in wastewater and even drinking water. Conventional wastewater treatment plants were not designed for the removal of these drug residues. For this reason, these micropollutants, which cannot be treated in wastewater treatment plants, are discharged to the receiving environment and cause negative effects there. Recently, advanced oxidation processes have been frequently used for the removal of such micropollutants. In this study, life cycle assessment (LCA) of two different advanced oxidation processes was carried out to determine the environmental effects of ibuprofen removal. CML 2 baseline method of SimaPro 8.0.2 software was used in the study. At the end of the study, the environmental impact of the UV/H2O2 process was found to be higher. It has been determined that the most important parameter that causes environmental impact is electrical energy consumption.

Kaynakça

  • Bello, M. M., Abdul Raman, A. A., & Asghar, A. (2019). A review on approaches for addressing the limitations of Fenton oxidation for recalcitrant wastewater treatment. Process Safety and Environmental Protection, 126, 119–140. https://doi.org/10.1016/j.psep.2019.03.028
  • Çatalkaya, E., Bali, U., & Şengül, F. (2004). Fenol’ün fotokimyasal yöntemlerle parçalanması ve mineralizasyonu. SKKD, 14(3), 31–41.
  • Çolak Güneş, N. (2020). Yaşam Döngüsü Analizi ile Konsantre Şeftali Püresinin Karbon Ayak İzinin Belirlenmesi. Akademik Gıda, 18(3), 247–255. https://doi.org/10.24323/akademik-gida.818098
  • De la Cruz, N., Giménez, J., Esplugas, S., Grandjean, D., De Alencastro, L. F., & Pulgarín, C. (2012). Degradation of 32 emergent contaminants by UV and neutral photo-fenton in domestic wastewater effluent previously treated by activated sludge. Water Research, 46(6), 1947–1957. https://doi.org/10.1016/j.watres.2012.01.014
  • Eren, Ö., & Öztürk, H. (2021). Tatlı Sorgum (Sorghum Bicolor (L)) Biyokütlesinin Yaşam Döngüsü Değerlendirmesi ile Çevresel Etkilerinin Belirlenmesi. European Journal of Science and Technology, (22), 195–203. https://doi.org/10.31590/ejosat.852286
  • García-Montaño, J., Ruiz, N., Muñoz, I., Domènech, X., García-Hortal, J. A., Torrades, F., & Peral, J. (2006). Environmental assessment of different photo-Fenton approaches for commercial reactive dye removal. Journal of Hazardous Materials, 138(2), 218–225. https://doi.org/10.1016/j.jhazmat.2006.05.061
  • Klavarioti, M., Mantzavinos, D., & Kassinos, D. (2009). Removal of residual pharmaceuticals from aqueous systems by advanced oxidation processes. Environment International, 35(2 Huang, C P, Dong, Chengdi, and Tang, Zhonghung. Advanced chemical oxidation: Its present role and potential future in hazardous waste treatment. United States: N. p., 1993. Web. doi:10.1016/0956-053X(93)90070-D.), 402–417. https://doi.org/10.1016/J.ENVINT.2008.07.009
  • Kristensen, D. M., Desdoits-Lethimonier, C., Mackey, A. L., Dalgaard, M. D., De Masi, F., Munkbøl, C. H., … Jégou, B. (2018). Ibuprofen alters human testicular physiology to produce a state of compensated hypogonadism. Proceedings of the National Academy of Sciences, 115(4), 715–724. https://doi.org/10.1073/pnas.1715035115
  • Luo, Y., Guo, W., Ngo, H. H., Nghiem, L. D., Hai, F. I., Zhang, J., … Wang, X. C. (2014). A review on the occurrence of micropollutants in the aquatic environment and their fate and removal during wastewater treatment. Science of The Total Environment, 473–474, 619–641. https://doi.org/10.1016/J.SCITOTENV.2013.12.065
  • Maryam, B., Buscio, V., Odabasi, S. U., & Buyukgungor, H. (2020). A study on behavior, interaction and rejection of Paracetamol, Diclofenac and Ibuprofen (PhACs) from wastewater by nanofiltration membranes. Environmental Technology and Innovation, 18, 100641. https://doi.org/10.1016/j.eti.2020.100641
  • Mathias, F. T., Fockink, D. H., Disner, G. R., Prodocimo, V., Ribas, J. L. C., Ramos, L. P., … Silva de Assis, H. C. (2018). Effects of low concentrations of ibuprofen on freshwater fish Rhamdia quelen. Environmental Toxicology and Pharmacology, 59, 105–113. https://doi.org/https://doi.org/10.1016/j.etap.2018.03.008
  • Merck. (2021). https://www.sigmaaldrich.com/TR/en erişim:13.10.2021
  • Mirzaei, A., Chen, Z., Haghighat, F., & Yerushalmi, L. (2017). Removal of pharmaceuticals from water by homo/heterogonous Fenton-type processes – A review. Chemosphere, 174, 665–688. https://doi.org/10.1016/j.chemosphere.2017.02.019
  • Moynan, A. B., & Welsh, C. A. (2012). The Photodegradation of Ibuprofen and Dissolved Organic Matter in Lake Superior and St. Louis River Water. Zebrafish, 9(4), 179–184. https://doi.org/10.1089/zeb.2012.0754
  • Pesqueira, J. F. J. R., Pereira, M. F. R., & Silva, A. M. T. (2021b). A life cycle assessment of solar-based treatments (H2O2, TiO2 photocatalysis, circumneutral photo-Fenton) for the removal of organic micropollutants. Science of the Total Environment, 761, 143258. https://doi.org/10.1016/j.scitotenv.2020.143258
  • Rekhate, C. V., & Srivastava, J. K. (2020). Recent advances in ozone-based advanced oxidation processes for treatment of wastewater- A review. Chemical Engineering Journal Advances, 3(June), 100031. https://doi.org/10.1016/j.ceja.2020.100031
  • Rodríguez, R., Espada, J. J., Pariente, M. I., Melero, J. A., Martínez, F., & Molina, R. (2016b). Comparative life cycle assessment (LCA) study of heterogeneous and homogenous Fenton processes for the treatment of pharmaceutical wastewater. Journal of Cleaner Production, 124, 21–29. https://doi.org/10.1016/j.jclepro.2016.02.064
  • Salihoğlu, G., Poroy, Z., & Salihoğlu, N. K. (2019). Life Cycle Assessment for Municipal Waste Management: Analysis for Bursa. Pamukkale University Journal of Engineering Sciences, 25(6), 692–699. https://doi.org/10.5505/pajes.2018.33603
  • Schwaiger, J., Ferling, H., Mallow, U., Wintermayr, H., & Negele, R. D. (2004). Toxic effects of the non-steroidal anti-inflammatory drug diclofenac: Part I: histopathological alterations and bioaccumulation in rainbow trout. Aquatic Toxicology, 68(2), 141–150. https://doi.org/https://doi.org/10.1016/j.aquatox.2004.03.014
  • Aydın, S. (2016). Pamuklu Ev Tekstil Ürünlerinin Üretim Süreçleri ve Nihai Ürünlerin Yaşam Döngüsünün Değerlendirilmesi. Yüksek Lisans Tezi, Niğde Ünversitesi, Fen Bilimleri Enstitüsü, Niğde.
  • Sönmez, G. (2015). İleri Oksidasyon Prosesleri ile Bazı İlaç Kalıntılarının Giderimi. Doktora Tezi, Aksaray Üniversitesi, Fen Bilimleri Enstitüsü, Aksaray.
  • TEIAS. (2021). https://www.tedas.gov.tr/#!tedas_tarifeler erişim: 13.10.2021
  • Üstün-Odabaşı, S., Maryam, B., Özdemir, N., & Büyükgüngör, H. (2020). Occurrence and seasonal variations of pharmaceuticals and personal care products in drinking water and wastewater treatment plants in Samsun, Turkey. Environmental Earth Sciences, 79(12). https://doi.org/10.1007/s12665-020-09047-7
  • Üstün Odabaşı, S., & Büyükgüngör, H. (2017). Investigation and Evaluation of Degradability of Ibuprofen from Wastewater by Using Fenton Process Publication Info Investigation and Evaluation of Degradability of Ibuprofen from Wastewater by Using Fenton Process. European Journal of Engineering and Natural Sciences, 2(1), 114–119.
  • Üstün Odabaşı, S., Maryam, B., & Büyükgüngör, H. (2018). Fenton Oxidation of Carbamazepine in Wastewater with Fewer Reagents. Sigma Journal of Engineering and Natural Sciences, 36(1), 289–298.

Ibuprofenin ileri oksidasyon prosesleri ile gideriminin yaşam döngüsü değerlendirmesi

Yıl 2021, Sayı: 28, 795 - 801, 30.11.2021

Öz

Steroid olmayan anti-inflamatuvar (NSAI) grubunda yer alan ibuprofen (IBU), atıksularda ve hatta içme sularında sıklıkla tespit edilmektedir. Klasik atıksu arıtma tesisleri bu ilaç kalıntılarının giderimi üzerine projelendirilmemiştir. Bu nedenle atıksu arıtma tesislerinde arıtılamayan bu mikrokirleticiler alıcı ortamlara deşaj edilmekte ve burada olumsuz etkilere neden olmaktadır. Son zamanlarda ileri oksidasyon prosesleri bu tarz mikrokirleticilerin gideriminde sıklıkla kullanılmaktadır. Bu çalışmada da ibuprofen gideriminin çevresel etkilerini belirlemek amacıyla iki farklı ileri oksidasyon prosesinin yaşam döngüsü değerlendirmesi (YDD) yapılmıştır. Çalışmada SimaPro 8.0.2 yazılımının CML 2 baseline metodu kullanılmıştır. Çalışma sonunda UV/H2O2 prosesinin çevresel etkisi daha yüksek bulunmuştur. Çevresel etkiye sebep olan en önemli parametre olarak ise elektrik enerjisi tüketimi olduğu tespit edilmiştir.

Kaynakça

  • Bello, M. M., Abdul Raman, A. A., & Asghar, A. (2019). A review on approaches for addressing the limitations of Fenton oxidation for recalcitrant wastewater treatment. Process Safety and Environmental Protection, 126, 119–140. https://doi.org/10.1016/j.psep.2019.03.028
  • Çatalkaya, E., Bali, U., & Şengül, F. (2004). Fenol’ün fotokimyasal yöntemlerle parçalanması ve mineralizasyonu. SKKD, 14(3), 31–41.
  • Çolak Güneş, N. (2020). Yaşam Döngüsü Analizi ile Konsantre Şeftali Püresinin Karbon Ayak İzinin Belirlenmesi. Akademik Gıda, 18(3), 247–255. https://doi.org/10.24323/akademik-gida.818098
  • De la Cruz, N., Giménez, J., Esplugas, S., Grandjean, D., De Alencastro, L. F., & Pulgarín, C. (2012). Degradation of 32 emergent contaminants by UV and neutral photo-fenton in domestic wastewater effluent previously treated by activated sludge. Water Research, 46(6), 1947–1957. https://doi.org/10.1016/j.watres.2012.01.014
  • Eren, Ö., & Öztürk, H. (2021). Tatlı Sorgum (Sorghum Bicolor (L)) Biyokütlesinin Yaşam Döngüsü Değerlendirmesi ile Çevresel Etkilerinin Belirlenmesi. European Journal of Science and Technology, (22), 195–203. https://doi.org/10.31590/ejosat.852286
  • García-Montaño, J., Ruiz, N., Muñoz, I., Domènech, X., García-Hortal, J. A., Torrades, F., & Peral, J. (2006). Environmental assessment of different photo-Fenton approaches for commercial reactive dye removal. Journal of Hazardous Materials, 138(2), 218–225. https://doi.org/10.1016/j.jhazmat.2006.05.061
  • Klavarioti, M., Mantzavinos, D., & Kassinos, D. (2009). Removal of residual pharmaceuticals from aqueous systems by advanced oxidation processes. Environment International, 35(2 Huang, C P, Dong, Chengdi, and Tang, Zhonghung. Advanced chemical oxidation: Its present role and potential future in hazardous waste treatment. United States: N. p., 1993. Web. doi:10.1016/0956-053X(93)90070-D.), 402–417. https://doi.org/10.1016/J.ENVINT.2008.07.009
  • Kristensen, D. M., Desdoits-Lethimonier, C., Mackey, A. L., Dalgaard, M. D., De Masi, F., Munkbøl, C. H., … Jégou, B. (2018). Ibuprofen alters human testicular physiology to produce a state of compensated hypogonadism. Proceedings of the National Academy of Sciences, 115(4), 715–724. https://doi.org/10.1073/pnas.1715035115
  • Luo, Y., Guo, W., Ngo, H. H., Nghiem, L. D., Hai, F. I., Zhang, J., … Wang, X. C. (2014). A review on the occurrence of micropollutants in the aquatic environment and their fate and removal during wastewater treatment. Science of The Total Environment, 473–474, 619–641. https://doi.org/10.1016/J.SCITOTENV.2013.12.065
  • Maryam, B., Buscio, V., Odabasi, S. U., & Buyukgungor, H. (2020). A study on behavior, interaction and rejection of Paracetamol, Diclofenac and Ibuprofen (PhACs) from wastewater by nanofiltration membranes. Environmental Technology and Innovation, 18, 100641. https://doi.org/10.1016/j.eti.2020.100641
  • Mathias, F. T., Fockink, D. H., Disner, G. R., Prodocimo, V., Ribas, J. L. C., Ramos, L. P., … Silva de Assis, H. C. (2018). Effects of low concentrations of ibuprofen on freshwater fish Rhamdia quelen. Environmental Toxicology and Pharmacology, 59, 105–113. https://doi.org/https://doi.org/10.1016/j.etap.2018.03.008
  • Merck. (2021). https://www.sigmaaldrich.com/TR/en erişim:13.10.2021
  • Mirzaei, A., Chen, Z., Haghighat, F., & Yerushalmi, L. (2017). Removal of pharmaceuticals from water by homo/heterogonous Fenton-type processes – A review. Chemosphere, 174, 665–688. https://doi.org/10.1016/j.chemosphere.2017.02.019
  • Moynan, A. B., & Welsh, C. A. (2012). The Photodegradation of Ibuprofen and Dissolved Organic Matter in Lake Superior and St. Louis River Water. Zebrafish, 9(4), 179–184. https://doi.org/10.1089/zeb.2012.0754
  • Pesqueira, J. F. J. R., Pereira, M. F. R., & Silva, A. M. T. (2021b). A life cycle assessment of solar-based treatments (H2O2, TiO2 photocatalysis, circumneutral photo-Fenton) for the removal of organic micropollutants. Science of the Total Environment, 761, 143258. https://doi.org/10.1016/j.scitotenv.2020.143258
  • Rekhate, C. V., & Srivastava, J. K. (2020). Recent advances in ozone-based advanced oxidation processes for treatment of wastewater- A review. Chemical Engineering Journal Advances, 3(June), 100031. https://doi.org/10.1016/j.ceja.2020.100031
  • Rodríguez, R., Espada, J. J., Pariente, M. I., Melero, J. A., Martínez, F., & Molina, R. (2016b). Comparative life cycle assessment (LCA) study of heterogeneous and homogenous Fenton processes for the treatment of pharmaceutical wastewater. Journal of Cleaner Production, 124, 21–29. https://doi.org/10.1016/j.jclepro.2016.02.064
  • Salihoğlu, G., Poroy, Z., & Salihoğlu, N. K. (2019). Life Cycle Assessment for Municipal Waste Management: Analysis for Bursa. Pamukkale University Journal of Engineering Sciences, 25(6), 692–699. https://doi.org/10.5505/pajes.2018.33603
  • Schwaiger, J., Ferling, H., Mallow, U., Wintermayr, H., & Negele, R. D. (2004). Toxic effects of the non-steroidal anti-inflammatory drug diclofenac: Part I: histopathological alterations and bioaccumulation in rainbow trout. Aquatic Toxicology, 68(2), 141–150. https://doi.org/https://doi.org/10.1016/j.aquatox.2004.03.014
  • Aydın, S. (2016). Pamuklu Ev Tekstil Ürünlerinin Üretim Süreçleri ve Nihai Ürünlerin Yaşam Döngüsünün Değerlendirilmesi. Yüksek Lisans Tezi, Niğde Ünversitesi, Fen Bilimleri Enstitüsü, Niğde.
  • Sönmez, G. (2015). İleri Oksidasyon Prosesleri ile Bazı İlaç Kalıntılarının Giderimi. Doktora Tezi, Aksaray Üniversitesi, Fen Bilimleri Enstitüsü, Aksaray.
  • TEIAS. (2021). https://www.tedas.gov.tr/#!tedas_tarifeler erişim: 13.10.2021
  • Üstün-Odabaşı, S., Maryam, B., Özdemir, N., & Büyükgüngör, H. (2020). Occurrence and seasonal variations of pharmaceuticals and personal care products in drinking water and wastewater treatment plants in Samsun, Turkey. Environmental Earth Sciences, 79(12). https://doi.org/10.1007/s12665-020-09047-7
  • Üstün Odabaşı, S., & Büyükgüngör, H. (2017). Investigation and Evaluation of Degradability of Ibuprofen from Wastewater by Using Fenton Process Publication Info Investigation and Evaluation of Degradability of Ibuprofen from Wastewater by Using Fenton Process. European Journal of Engineering and Natural Sciences, 2(1), 114–119.
  • Üstün Odabaşı, S., Maryam, B., & Büyükgüngör, H. (2018). Fenton Oxidation of Carbamazepine in Wastewater with Fewer Reagents. Sigma Journal of Engineering and Natural Sciences, 36(1), 289–298.
Toplam 25 adet kaynakça vardır.

Ayrıntılar

Birincil Dil Türkçe
Konular Mühendislik
Bölüm Makaleler
Yazarlar

Sevde Ustun Odabasi 0000-0003-3533-4089

Yayımlanma Tarihi 30 Kasım 2021
Yayımlandığı Sayı Yıl 2021 Sayı: 28

Kaynak Göster

APA Ustun Odabasi, S. (2021). Ibuprofenin ileri oksidasyon prosesleri ile gideriminin yaşam döngüsü değerlendirmesi. Avrupa Bilim Ve Teknoloji Dergisi(28), 795-801. https://doi.org/10.31590/ejosat.1011436