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ADSORPSİYON PROSESİNİN NANO SIFIR DEĞERLİ DEMİR PARÇACIKLARI (NZVI) YOLUYLA ÇÖP SIZINTI SUYU ARITIMI

Year 2024, , 896 - 907, 03.09.2024

Serdar Göçer , Zeynep Zaimoğlu , Kevser Cırık

https://doi.org/10.17780/ksujes.1435586

Abstract

Çöp sızıntı suyu (LFL), kirletici maddelerin karmaşıklığı ve çeşitliliği nedeniyle önemli bir çevresel tehdittir. LFL arıtımı için önerilen çeşitli fiziksel, kimyasal ve biyolojik arıtma yöntemleri bulunmaktadır. Manyetik nanopartiküller, geleneksel adsorbanlarla karşılaştırıldığında başarılı etkiye sahip, yaygın olarak kullanılan adsorbanlardır. Manyetik adsorbanlar, uygun stabiliteye, yüksek adsorpsiyon kapasitesine, yüksek giderim verimliliğine ve yeniden kullanılabilirlik özelliklerine sahip adsorbanlardır. Nano sıfır değerlikli demir (SDD), atık sularda, özellikle de LFL' de bulunan kirletici maddeleri gidermek için etkili bir adsorbandır. Bu çalışmada LFL ön arıtımında nZVI kullanılmıştır. Adsorpsiyon çalışmasında, 50'den 500 mg nZVI/L' ye artan konsantrasyonlarda, 3'ten 8'e pH' larda ve 15'ten 330 dakikaya kadar temas sürelerinde test edilmiştir. Sistem performansı, çöp sızıntı suyunda bulunan Kimyasal Oksijen İhtiyacı (KOİ), Çözünmüş Organik Karbon (ÇOK), Toplam Azot (TN), Nitrat (NO3-) ve Amonyum (NH4+) gibi çeşitli kirletici parametrelerle değerlendirilmiştir. Çalışma sonunda elde edilen giderim verimleri sırasıyla %60, %60, %74, %56 ve %33 olarak belirlenmiştir. Sonuç olarak LFL' nin nZVI kullanılarak adsorpsiyon prosesi ile arıtılması için optimum koşullar 50 mg nZVI/L, pH 8 ve temas süresi 120 dakika olarak belirlenmiştir.

Keywords

Sıfır değerlikli demir Çöp Sızıntı Suları Adsorpsiyon Prosesi Manyetik Adsorbanlar

References

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LANDFILL LEACHATE TREATMENT VIA NANO ZERO VALENT IRON PARTICLES (nZVI) OF ADSORPTION PROCESS

Year 2024, , 896 - 907, 03.09.2024

Serdar Göçer , Zeynep Zaimoğlu , Kevser Cırık

https://doi.org/10.17780/ksujes.1435586

Abstract

Landfill leachate (LFL) is a significant environmental threat due to the complexity and diversity of contaminants. There are various physical, chemical, and biological treatment methods recommended for LFL treatment. Magnetic nanoparticles are widely used adsorbents with a successful effect compared to traditional adsorbents. Magnetic adsorbents are adsorbents with suitable stability, high adsorption capacity, high removal efficiency, and reusable capabilities. Nano zero-valent iron (nZVI) is an effective adsorbent to remove contaminants found in wastewater, especially LFL. In this study, nZVI was used in the LFL pretreatment. In the adsorption study, it was tested at increasing concentrations from 50 to 500mg nZVI/L, pHs from 3 to 8, and contact times from 15 to 330 minutes. System performance was evaluated with various pollutant parameters such as chemical oxygen demand (COD), dissolved organic carbon (DOC), total nitrogen (TN), nitrate (NO3-), and ammonium (NH4+) found in garbage leachate. The removal efficiencies obtained at the end of the study were determined as 60%, 60%, 74%, 56% and 33%, respectively. As a result, the optimum conditions for the treatment of LFL by adsorption process using nZVI were determined as 50 mg nZVI/L, pH 8, and contact time 120 minutes.

Keywords

Zero Valent İron Landfill Leachate Adsorption Process Magnetic Adsorbent

References

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  • Atmaca, E. (2009). Treatment of landfill leachate by using electro-Fenton method. J Hazard Mater, 163(1):109–114. https://doi.org/10.1016/j.jhazmat.2008.06.067.
  • Augusto, P.A., Castelo-Grande, T., Merchan, L., Estevez, A.M., Quintero, X., & Barbosa, D. (2019). Landfill leachate treatment by sorption in magnetic particles: preliminary study. Science of the Total Environment, 648, 636-668. https://doi.org/10.1016/j.scitotenv.2018.08.056.
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  • Bhatt, A.H., Karanjekar, RV., Altouqi, S., Sattler, M.L., Hossain, M.S., & Chen, V.P. (2017). Estimating landfill leachate BOD and COD based on rainfall, ambient temperature, and waste composition: Exploration of a MARS statistical approach. Environmental Technology & Innovation, 8, 1-16. https://doi.org/10.1016/j.eti.2017.03.003.
  • Brasil, Y.L., Silva, A.F., Gomes, R. F., & Amaral, M.C. (2021). Technical and economic evaluation of the integration of membrane bioreactor and air-stripping/absorption processes in the treatment of landfill leachate. Waste Management, 134, 110-119. https://doi.org/10.1016/j.wasman.2021.08.013.
  • Brennan, R.B., Healy, M.G., Morrison, L., Hynes, S., Norton, D., & Clifford, E. (2016). Management of landfill leachate: The legacy of European Union Directives. Waste management, 55, 355-363. https://doi.org/10.1016/j.wasman.2015.10.010.
  • Chang, Y.C., & Chen, D.H. (2005). Preparation and adsorption properties of monodisperse chitosan-bound Fe3O4 magnetic nanoparticles for removal of Cu (II) ions. Journal of colloid and interface science, 283(2), 446-451. https://doi.org/10.1016/j.jcis.2004.09.010.
  • Chen, Z., Wang, X., Yang, Y., Mirino Jr, M.W., & Yuan, Y. (2016). Partial nitrification and denitrification of mature landfill leachate using a pilot-scale continuous activated sludge process at low dissolved oxygen. Bioresource technology, 218, 580-588. https://doi.org/10.1016/j.biortech.2016.07.008.
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  • Foo, K.Y., & Hameed, B. H. (2009). An overview of landfill leachate treatment via activated carbon adsorption process. Journal of hazardous materials, 171(1-3), 54-60. https://doi.org/10.1016/j.jhazmat.2009.06.038.
  • Fu, F., Dionysiou, D. D., & Liu, H. (2014). The use of zero-valent iron for groundwater remediation and wastewater treatment: a review. Journal of hazardous materials, 267, 194-205. https://doi.org/10.1016/j.jhazmat.2013.12.062.
  • Gajski, G., Oreščanin, V & Garaj-Vrhovac, V. (2012). Chemical composition and genotoxicity assessment of sanitary landfill leachate from Rovinj, Croatia. Ecotoxicology and environmental safety, 78, 253-259. https://doi.org/10.1016/j.ecoenv.2011.11.032.
  • Galdames, A., Ruiz-Rubio, L., Orueta, M., Sánchez-Arzalluz, M., & Vilas-Vilela, J.L. (2020). Zero-valent iron nanoparticles for soil and groundwater remediation. International Journal of Environmental Research and Public Health, 17(16), 5817. https://doi.org/10.3390/ijerph17165817.
  • Ghasemzadeh, G., Momenpour, M., Omidi, F., Hosseini, M.R., Ahani, M., & Barzegari, A. (2014). Applications of nanomaterials in water treatment and environmental remediation. Frontiers of environmental science & engineering, 8, 471-482. https://doi.org/10.1007/s11783-014-0654-0.
  • Göçer S., Kozak M., Akgül V., Duyar A., Zaimoğlu Z. &Cırık K. (2019) Synthesıs Of Nanoscale Zero-Valent Iron (nZVI), International Symposium on Advanced Engineering Technologies (ISADET), 02-04 May 2019, p:828-833, Kahramanmaraş/Turkey.
  • Göçer, S., Zaimoğlu, B. Z., & Cırık, K. (2024). Removal of pollutants from landfill leachate by adsorption with nano zero-valent iron particles: adsorption isotherms and kinetic studies. Water Practice & Technology, 19(2), 401-418. https://doi.org/10.2166/wpt.2024.029.
  • Gotvajn AZ, Tisler T. & Zagorc-Koncan J. (2009). Comparison of different treatment strategies for industrial landfill leachate. J Hazard Mater, 162(2–3):1446–1456. https://doi.org/10.1016/j.jhazmat.2008.06.037.
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There are 54 citations in total.

Details

Primary Language English
Subjects Environmental Engineering (Other)
Journal Section Environmental Engineering
Authors

Serdar Göçer 0000-0003-0443-8045

Zeynep Zaimoğlu 0000-0002-9573-4781

Kevser Cırık 0000-0002-1756-553X

Publication Date September 3, 2024
Submission Date February 12, 2024
Acceptance Date May 15, 2024
Published in Issue Year 2024

Cite

APA Göçer, S., Zaimoğlu, Z., & Cırık, K. (2024). LANDFILL LEACHATE TREATMENT VIA NANO ZERO VALENT IRON PARTICLES (nZVI) OF ADSORPTION PROCESS. Kahramanmaraş Sütçü İmam Üniversitesi Mühendislik Bilimleri Dergisi, 27(3), 896-907. https://doi.org/10.17780/ksujes.1435586